Combine 2 cups flour and sugar in a large mixing bowl. Cut in butter until mixture resembles coarse meal. Set aside 3/4 cup crumb mixture. Combine remaining crumb mixture and 1/3 cup flour. Add egg, buttermilk, soda, and cinnamon; stir until moistened. Pour batter into a greased 9-inch square pan. Combine reserved crumb mixture with nuts; sprinkle over batter. Bake at 325°F for 1 hour or until coffee cake tests done. Cut into squares.
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